You can do this by visiting your account settings page and clicking on the Subscription link there. Then scroll down...

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Source: http://silversingles-support.bravesites.com/entries/general/How-Do-I-Cancel-My-POF-Subscription-On-iPhone-

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You can do this by visiting your account settings page and clicking on the Subscription link there. Then scroll down to Cancel Subscription and follow the instructions from there. To get started canceling your POF subscription from your iPhone today just follow these steps:

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